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2.
Environ Sci Technol ; 55(24): 16573-16580, 2021 12 21.
Artigo em Inglês | MEDLINE | ID: mdl-34842427

RESUMO

Two years of satellite observations were used to quantify methane emissions from coal mines in Queensland, the largest coal-producing state in Australia. The six analyzed surface and underground coal mines are estimated to emit 570 ± 98 Gg a-1 in 2018-2019. Together, they account for 7% of the national coal production while emitting 55 ± 10% of the reported methane emission from coal mining in Australia. Our results indicate that for two of the three locations, our satellite-based estimates are significantly higher than reported to the Australian government. Most remarkably, 40% of the quantified emission came from a single surface mine (Hail Creek) located in a methane-rich coal basin. Our findings call for increased monitoring and investment in methane recovery technologies for both surface and underground mines.


Assuntos
Minas de Carvão , Metano , Austrália , Carvão Mineral , Metano/análise
3.
Nature ; 597(7876): 366-369, 2021 09.
Artigo em Inglês | MEDLINE | ID: mdl-34526704

RESUMO

Southeast Australia experienced intensive and geographically extensive wildfires during the 2019-2020 summer season1,2. The fires released substantial amounts of carbon dioxide into the atmosphere3. However, existing emission estimates based on fire inventories are uncertain4, and vary by up to a factor of four for this event. Here we constrain emission estimates with the help of satellite observations of carbon monoxide5, an analytical Bayesian inversion6 and observed ratios between emitted carbon dioxide and carbon monoxide7. We estimate emissions of carbon dioxide to be 715 teragrams (range 517-867) from November 2019 to January 2020. This is more than twice the estimate derived by five different fire inventories8-12, and broadly consistent with estimates based on a bottom-up bootstrap analysis of this fire episode13. Although fires occur regularly in the savannas in northern Australia, the recent episodes were extremely large in scale and intensity, burning unusually large areas of eucalyptus forest in the southeast13. The fires were driven partly by climate change14,15, making better-constrained emission estimates particularly important. This is because the build-up of atmospheric carbon dioxide may become increasingly dependent on fire-driven climate-carbon feedbacks, as highlighted by this event16.


Assuntos
Dióxido de Carbono/análise , Imagens de Satélites , Incêndios Florestais/estatística & dados numéricos , Atmosfera/química , Austrália , Teorema de Bayes , Monóxido de Carbono/análise , Mudança Climática , Eucalyptus , Florestas , Pradaria , Incerteza
4.
Sci Rep ; 11(1): 4138, 2021 02 18.
Artigo em Inglês | MEDLINE | ID: mdl-33602990

RESUMO

Quantifying natural geological sources of methane (CH4) allows to improve the assessment of anthropogenic emissions to the atmosphere from fossil fuel industries. The global CH4 flux of geological gas is, however, an object of debate. Recent fossil (14C-free) CH4 measurements in preindustrial-era ice cores suggest very low global geological emissions (~ 1.6 Tg year-1), implying a larger fossil fuel industry source. This is however in contrast with previously published bottom-up and top-down geo-emission estimates (~ 45 Tg year-1) and even regional-scale emissions of ~ 1-2 Tg year-1. Here we report on significant geological CH4 emissions from the Lusi hydrothermal system (Indonesia), measured by ground-based and satellite (TROPOMI) techniques. Both techniques indicate a total CH4 output of ~ 0.1 Tg year-1, equivalent to the minimum value of global geo-emission derived by ice core 14CH4 estimates. Our results are consistent with the order of magnitude of the emission factors of large seeps used in global bottom-up estimates, and endorse a substantial contribution from natural Earth's CH4 degassing. The preindustrial ice core assessments of geological CH4 release may be underestimated and require further study. Satellite measurements can help to test geological CH4 emission factors and explain the gap between the contrasting estimates.

5.
Sci Adv ; 6(17): eaaz5120, 2020 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-32494644

RESUMO

Using new satellite observations and atmospheric inverse modeling, we report methane emissions from the Permian Basin, which is among the world's most prolific oil-producing regions and accounts for >30% of total U.S. oil production. Based on satellite measurements from May 2018 to March 2019, Permian methane emissions from oil and natural gas production are estimated to be 2.7 ± 0.5 Tg a-1, representing the largest methane flux ever reported from a U.S. oil/gas-producing region and are more than two times higher than bottom-up inventory-based estimates. This magnitude of emissions is 3.7% of the gross gas extracted in the Permian, i.e., ~60% higher than the national average leakage rate. The high methane leakage rate is likely contributed by extensive venting and flaring, resulting from insufficient infrastructure to process and transport natural gas. This work demonstrates a high-resolution satellite data-based atmospheric inversion framework, providing a robust top-down analytical tool for quantifying and evaluating subregional methane emissions.

6.
Proc Natl Acad Sci U S A ; 116(52): 26376-26381, 2019 Dec 26.
Artigo em Inglês | MEDLINE | ID: mdl-31843920

RESUMO

Methane emissions due to accidents in the oil and natural gas sector are very challenging to monitor, and hence are seldom considered in emission inventories and reporting. One of the main reasons is the lack of measurements during such events. Here we report the detection of large methane emissions from a gas well blowout in Ohio during February to March 2018 in the total column methane measurements from the spaceborne Tropospheric Monitoring Instrument (TROPOMI). From these data, we derive a methane emission rate of 120 ± 32 metric tons per hour. This hourly emission rate is twice that of the widely reported Aliso Canyon event in California in 2015. Assuming the detected emission represents the average rate for the 20-d blowout period, we find the total methane emission from the well blowout is comparable to one-quarter of the entire state of Ohio's reported annual oil and natural gas methane emission, or, alternatively, a substantial fraction of the annual anthropogenic methane emissions from several European countries. Our work demonstrates the strength and effectiveness of routine satellite measurements in detecting and quantifying greenhouse gas emission from unpredictable events. In this specific case, the magnitude of a relatively unknown yet extremely large accidental leakage was revealed using measurements of TROPOMI in its routine global survey, providing quantitative assessment of associated methane emissions.

7.
Nat Commun ; 8(1): 2227, 2017 12 20.
Artigo em Inglês | MEDLINE | ID: mdl-29263323

RESUMO

Several viable but conflicting explanations have been proposed to explain the recent ~8 p.p.b. per year increase in atmospheric methane after 2006, equivalent to net emissions increase of ~25 Tg CH4 per year. A concurrent increase in atmospheric ethane implicates a fossil source; a concurrent decrease in the heavy isotope content of methane points toward a biogenic source, while other studies propose a decrease in the chemical sink (OH). Here we show that biomass burning emissions of methane decreased by 3.7 (±1.4) Tg CH4 per year from the 2001-2007 to the 2008-2014 time periods using satellite measurements of CO and CH4, nearly twice the decrease expected from prior estimates. After updating both the total and isotopic budgets for atmospheric methane with these revised biomass burning emissions (and assuming no change to the chemical sink), we find that fossil fuels contribute between 12-19 Tg CH4 per year to the recent atmospheric methane increase, thus reconciling the isotopic- and ethane-based results.

8.
Sci Rep ; 7: 45759, 2017 04 10.
Artigo em Inglês | MEDLINE | ID: mdl-28393869

RESUMO

Year-to-year variations in the atmospheric methane (CH4) growth rate show significant correlation with climatic drivers. The second half of 2010 and the first half of 2011 experienced the strongest La Niña since the early 1980s, when global surface networks started monitoring atmospheric CH4 mole fractions. We use these surface measurements, retrievals of column-averaged CH4 mole fractions from GOSAT, new wetland inundation estimates, and atmospheric δ13C-CH4 measurements to estimate the impact of this strong La Niña on the global atmospheric CH4 budget. By performing atmospheric inversions, we find evidence of an increase in tropical CH4 emissions of ∼6-9 TgCH4 yr-1 during this event. Stable isotope data suggest that biogenic sources are the cause of this emission increase. We find a simultaneous expansion of wetland area, driven by the excess precipitation over the Tropical continents during the La Niña. Two process-based wetland models predict increases in wetland area consistent with observationally-constrained values, but substantially smaller per-area CH4 emissions, highlighting the need for improvements in such models. Overall, tropical wetland emissions during the strong La Niña were at least by 5% larger than the long-term mean.

10.
Nature ; 456(7222): 628-30, 2008 Dec 04.
Artigo em Inglês | MEDLINE | ID: mdl-19052625

RESUMO

Terrestrial wetland emissions are the largest single source of the greenhouse gas methane. Northern high-latitude wetlands contribute significantly to the overall methane emissions from wetlands, but the relative source distribution between tropical and high-latitude wetlands remains uncertain. As a result, not all the observed spatial and seasonal patterns of atmospheric methane concentrations can be satisfactorily explained, particularly for high northern latitudes. For example, a late-autumn shoulder is consistently observed in the seasonal cycles of atmospheric methane at high-latitude sites, but the sources responsible for these increased methane concentrations remain uncertain. Here we report a data set that extends hourly methane flux measurements from a high Arctic setting into the late autumn and early winter, during the onset of soil freezing. We find that emissions fall to a low steady level after the growing season but then increase significantly during the freeze-in period. The integral of emissions during the freeze-in period is approximately equal to the amount of methane emitted during the entire summer season. Three-dimensional atmospheric chemistry and transport model simulations of global atmospheric methane concentrations indicate that the observed early winter emission burst improves the agreement between the simulated seasonal cycle and atmospheric data from latitudes north of 60 degrees N. Our findings suggest that permafrost-associated freeze-in bursts of methane emissions from tundra regions could be an important and so far unrecognized component of the seasonal distribution of methane emissions from high latitudes.


Assuntos
Atmosfera/química , Congelamento , Metano/metabolismo , Áreas Alagadas , Regiões Árticas , Clima Frio , Groenlândia , Metano/análise , Estações do Ano , Solo/análise
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